Home To The Largest Urban Zoo In The United States With The Crossword Clue — 5 Letters

One confident answer with explanation of the wordplay

BRONX
Best match
B
R
O
N
X

The Bronx Zoo in New York City is widely recognized as the largest urban zoo in the United States. The clue specifies "with 'the'" because the borough is properly called "The Bronx."

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Other possible answers
INDIADelhi Zoo is large but not in the US
MIAMIZoo Miami is large but not typically cited as the largest urban zoo
OMAHAHenry Doorly Zoo is considered world-class but Omaha is not the standard answer for largest urban zoo

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